Conjugation & Pericyclic Reactions · Section 52 of 116

UV-Vis spectroscopy

Practice this — interactive lesson

Every other spectroscopy in this course reports on individual bonds or individual nuclei. UV-Vis reports on something more specific and more useful in this chapter: how far a conjugated π system extends. It is the experimental measurement of the thing the rest of this chapter has been reasoning about.

What the measurement is

Ultraviolet and visible light carry enough energy to promote an electron from an occupied molecular orbital to an empty one. In an organic molecule with a π system, the transition that matters is from the HOMO (highest occupied molecular orbital) to the LUMO (lowest unoccupied one) — a π → π* transition.

A molecule absorbs the wavelength whose photon energy matches that gap. Since energy and wavelength are inversely related, the relationship you actually use is short and worth memorizing in this direction:

Bigger HOMO–LUMO gap → higher energy photon needed → shorter wavelength absorbed.
Smaller gap → lower energy → longer wavelength absorbed.

More conjugation, smaller gap, longer wavelength

Extending a conjugated system adds more p orbitals to the combination, which produces more molecular orbitals, spread over a similar total energy range. The result is that the highest occupied one rises and the lowest empty one falls, so the gap between them narrows with every double bond added to the conjugation.

The numbers make the trend unmistakable, and they are worth knowing as a shape rather than as figures to recall exactly:

CompoundConjugated C=Cλmax (approx.)
Ethene1171 nm
Buta-1,3-diene2217 nm
Hexa-1,3,5-triene3258 nm
β-Carotene11~450 nm

The group responsible for the absorption is called a chromophore. An isolated C=C absorbs below about 200 nm, which is inconveniently far into the ultraviolet for ordinary instruments, so a simple alkene is effectively invisible. Conjugate two and the absorption moves into the accessible range — which is precisely why this technique is a conjugation detector rather than a general-purpose one.

Why conjugation eventually produces color

150200250300350400450500wavelength absorbed, λₘₐₓ (nm)Ethene171 nm1 conjugated C=CButa-1,3-diene217 nm2Hexa-1,3,5-triene258 nm3β-Carotene450 nm11out of rangevisible regiona lone C=C absorbs herehere the compound has a colorEach double bond added to the conjugation narrows the gap, so λₘₐₓ moves right.
The four compounds from the table, placed on the axis they actually differ along. An isolated double bond absorbs off the left-hand end of the accessible range; each double bond joined to the conjugation moves the absorption to the right, and with eleven of them β-carotene has walked all the way into visible light.The two shaded bands are why this technique is a conjugation detector rather than a general one. Below about 200 nm an ordinary instrument cannot look, so a lone alkene is invisible; past 400 nm the molecule is removing visible light and the compound has a color — β-carotene absorbs blue near 450 nm, which is why what reaches your eye is orange. A colorless organic compound is a compound whose π system stopped short of the right-hand band.

Keep extending the system and λmax keeps rising until it crosses about 400 nm and enters the visible region. At that point the compound is absorbing visible light, and what your eye sees is the light that was not absorbed — the complementary color.

β-Carotene, with eleven conjugated double bonds, absorbs blue light around 450 nm and therefore looks orange. That is the color of carrots, and the same reasoning covers the deep colors of dyes, indicators and the visual pigment retinal. Organic compounds are colorless unless they carry an extensively conjugated system; when you see a strongly colored organic compound, extended conjugation is the first thing to look for.

Other structural features shift λmax in the same direction as extra conjugation — alkyl substituents on the π system, and lone pairs able to conjugate into it, both push it to longer wavelength. The effect is smaller than adding a whole double bond, but it is systematic enough that empirical rules exist to predict λmax for substituted dienes and enones.

Beer–Lambert: how much is absorbed

Wavelength says what the molecule is; the amount of absorption says how much of it is there. The relationship is the Beer–Lambert law:

A = εcl

Because absorbance is directly proportional to concentration, UV-Vis is a quantitative technique in a way NMR and IR usually are not in a teaching lab. It is the standard way to follow the concentration of a colored or conjugated species while a reaction runs.

Worked example — reading a spectrum

Two isomeric dienes, C₆H₁₀. One absorbs at 227 nm, the other below 200 nm. Which is conjugated?

The one at 227 nm. A conjugated diene has the smaller HOMO–LUMO gap and therefore absorbs at the longer wavelength. The isolated diene behaves as two separate alkenes, each absorbing below 200 nm where a simple C=C does.

What the spectrum does not tell you is where the double bonds are, only that they are or are not in conjugation. Pair it with NMR to place them — UV-Vis answers one question, sharply, and says little about anything else.

What carries forward

UV-Vis sits in this chapter rather than with IR and NMR on purpose: it is the direct measurement of conjugation, and it makes the abstract claim of the first section — that a longer π system is a lower-energy, smaller-gap system — into something you can read off an instrument. When you reach the Spectroscopy chapter, the habit to carry in is that each technique answers a different question: IR names functional groups, mass spectrometry gives mass and fragments, NMR builds the carbon skeleton, and UV-Vis reports conjugation.