Conjugation & Pericyclic Reactions · Section 51 of 116

The Diels–Alder reaction

Practice this — interactive lesson

The Diels–Alder reaction builds a six-membered ring in one step, from two pieces, with no intermediate, no catalyst and complete control of the stereochemistry. It is the most useful single reaction in this course and one of the most useful in organic chemistry generally, and almost everything about it follows from one picture: six electrons moving round a circle.

What it is

A conjugated diene (four π electrons) reacts with an alkene or alkyne called the dienophile — literally "diene-loving" — (two π electrons) to give a cyclohexene. Because it joins a four-π-electron component to a two-π-electron one, it is classified as a [4+2] cycloaddition.

The arithmetic of the bonds explains why it is so favorable. Three π bonds go in; out come two new σ bonds and one π bond. σ bonds are stronger than π bonds, so trading two of the latter for two of the former releases energy, and the reaction is downhill without anything having to drive it.

It is concerted: every bond breaks and forms in the same step, through a single cyclic transition state, with no intermediate at all. There is no carbocation, so there are no rearrangements, and there is nothing whose stability you need to compare. Almost every special property below is a consequence of that one fact.

The diene must be able to reach s-cis

diene, held s-cisC1C2C3C4dienophileone stepthe new π bond, C2 to C3C1C2C3C4the two new σ bondsThree π bonds in; two σ bonds and one π bond out — so it runs downhill unaided.
The whole reaction as one circle of six electrons. The diene’s C1 and C4 reach the two ends of the dienophile, the arrows chase each other head to tail round the ring, and every bond that breaks and every bond that forms does so in the same instant.Keep the numbering in view and the product is never a guess. C1 and C4 are where the new single bonds appear, so the new double bond has nowhere to be except between C2 and C3 — the bond that was single in the starting diene. And because the two new bonds form at once on one face of the dienophile, nothing has a chance to rotate in between, which is where the stereospecificity below comes from.

For the two ends of the diene to reach the two ends of the dienophile at the same time, they have to be on the same side — the diene must react from its s-cis conformation. This is the commonest reason a Diels–Alder simply does not happen, and it is a geometric requirement rather than an electronic one.

Electronics: electron-rich diene, electron-poor dienophile

The reaction is fastest when the two partners are electronically mismatched in the right direction. Electron-donating groups on the diene raise its HOMO; electron-withdrawing groups on the dienophile lower its LUMO. Bringing those two orbitals closer in energy makes the interaction between them stronger and the reaction faster.

In practice this means a good dienophile carries a carbonyl, a nitrile, a nitro group or an ester next to its double bond. Maleic anhydride, with two carbonyls flanking the alkene, is the classic fast dienophile; ethene itself reacts only under forcing conditions because it has nothing pulling its LUMO down.

Stereochemistry, and why it is completely predictable

Because the reaction is concerted, the geometry of the starting materials is carried straight into the product. Three separate statements follow, and they are the reason the reaction is so heavily used in synthesis.

It is stereospecific with respect to the dienophile. Both new bonds form on the same face of the dienophile, so substituents that were cis across its double bond come out cis on the ring, and trans comes out trans. There is no step at which anything can rotate.

The diene's geometry is carried through too. Groups at the diene's outer positions that pointed "outward" in the s-cis conformation end up on one face of the new ring, and those that pointed "inward" end up on the other.

The endo product is favored. When the dienophile carries a substituent, the two partners can stack in two orientations: endo, with the dienophile's substituent tucked under the diene, or exo, with it pointing away. The endo arrangement is more crowded and is nevertheless the faster one, because the substituent's π system interacts favorably with the developing π system of the diene in the transition state — a secondary orbital interaction. Endo is therefore the kinetic product, which is worth noticing: it is a case where the kinetic product is the more hindered one, and the general rule from the last section still holds because nothing here is reversing at ordinary temperatures.

Worked example — predicting a product completely

React buta-1,3-diene with dimethyl maleate, in which the two ester groups are cis across the double bond.

Skeleton. [4+2] gives a cyclohexene. The new double bond sits between what were C2 and C3 of the diene, and the two new σ bonds join the diene's C1 and C4 to the two dienophile carbons.

Stereochemistry. The two esters were cis on the dienophile, and the addition is suprafacial on it, so they are cis on the ring — on adjacent carbons, on the same face.

Check by switching. Run the same reaction with dimethyl fumarate, the trans isomer, and the two esters come out trans on the ring. One change in the starting material, one predictable change in the product, and no mixture in either case.

Running it backwards

The reaction is reversible, and heating a cyclohexene of the right kind drives the retro-Diels–Alder, splitting it back into a diene and a dienophile. Cracking cyclopentadiene dimer before use is exactly this. It also matters in synthesis planning: seeing a cyclohexene ring and mentally cutting it apart at the retro-Diels–Alder disconnection is one of the most productive moves available when you are working a synthesis backwards.

What carries forward

Three things. The Diels–Alder is the first concerted reaction in this course that forms two bonds at once, and the reasoning — frontier orbitals, suprafacial addition, stereospecificity — is the template for pericyclic chemistry generally. It is the standard way to make a six-membered ring, which makes it a fixture of retrosynthesis. And the endo rule is a clean reminder that "more stable" and "forms faster" are separate questions, which is the lesson of the section before this one.