Oxidation & Reduction · Section 65 of 116

Oxidative cleavage & dihydroxylation

Practice this — interactive lesson

The reactions in this section all oxidize a carbon–carbon double bond, and they differ in how far they go. One adds a single oxygen, one adds two hydroxyls, and one cuts the molecule in half. Choosing between them is choosing how much of the alkene you want left.

Epoxidation: one oxygen, ring intact

mCPBA (meta-chloroperoxybenzoic acid) delivers a single oxygen atom across the double bond to give an epoxide. The reaction is concerted — the oxygen is transferred in one step through a cyclic transition state — so it is stereospecific: a cis alkene gives the cis-substituted epoxide and a trans alkene gives the trans one, cleanly.

Epoxides are useful precisely because they are strained and therefore reactive, which is the subject of their own section in the alcohols chapter. Here the point is what happens when you open one with water.

The two diols, and how to choose between them

A 1,2-diol (a glycol) can be made from an alkene in two ways, and they give opposite stereochemistry. This is the most examinable fact in the section.

OsO₄ → syn diol. Epoxidation then hydrolysis → anti diol. Same starting alkene, same molecular formula in the product, different diastereomer. If a question specifies which diol it wants, it is testing exactly this pair.

Ozonolysis: cutting the double bond in half

one alkeneRHRHOsO₄, then NaHSO₃one cyclic osmate ester, so bothoxygens are delivered at oncemCPBA, then H₃O⁺the epoxide is opened by attackfrom the opposite faceRROHOHHHRROHOHHHsyn (cis) diolanti (trans) diolboth OH toward the reader — same faceone wedge, one hash — opposite faces
One alkene, two diols, and the same molecular formula in both products. The only difference is which face each hydroxyl arrived on — osmium delivers both oxygens together from one face, while the epoxide route delivers the second one from the other side.Read it off the wedges rather than off the names. Osmium tetroxide forms a five-membered osmate ester spanning both carbons, so the two oxygens are tied to the same face before the ring is ever cut off; there is no step at which they could end up anywhere else. Epoxidation then hydrolysis has an extra step, and that step is what flips the answer: water attacks the protonated epoxide from the side opposite the C–O bond that is breaking, which is the same backside attack an SN2 makes.

Ozone (O₃) cleaves a C=C completely, breaking both the σ and the π bond and leaving two separate carbonyl fragments. The workup then decides what those fragments are:

Hot, concentrated, acidic KMnO₄ does the same cleavage with the oxidative outcome, and is sometimes written in place of ozonolysis with peroxide workup.

Ozonolysis is a structure-determination tool as much as a synthesis one. Run it on an unknown alkene, identify the two carbonyl fragments, and mentally rejoin them at their carbonyl carbons — that reconstructs where the double bond was. Questions that give you the fragments and ask for the starting alkene are asking you to run exactly that reasoning backwards.
Worked example — reading a cleavage backwards

An unknown alkene C₆H₁₂ is ozonolyzed with Me₂S workup, giving propanal and propanone (acetone).

Rejoin at the carbonyl carbons. Propanal is CH₃CH₂CHO, so that carbon carried one hydrogen and an ethyl group. Propanone is (CH₃)₂CO, so that carbon carried two methyls.

Rebuild the double bond between those two carbons: CH₃CH₂–CH=C(CH₃)₂, which is 2-methylpent-2-ene. Check the formula: C₆H₁₂. ✓

The tell in the question is that one fragment is an aldehyde and one a ketone, which immediately says the original alkene was trisubstituted — one carbon bore a hydrogen, the other did not.

The whole section as one decision

ReagentWhat happens to the C=CProduct
mCPBAOne O added, ring keptEpoxide (stereospecific)
OsO₄ / NMOTwo OH, same facesyn diol
mCPBA then H₃O⁺Two OH, opposite facesanti diol
O₃ then Me₂SCleavedAldehydes and/or ketones
O₃ then H₂O₂CleavedCarboxylic acids and/or ketones
KMnO₄, hot/conc.CleavedCarboxylic acids and/or ketones
KMnO₄, cold/dilute/basicTwo OH, same facesyn diol

KMnO₄ appears twice on purpose, and the conditions are doing all the work: cold and dilute it stops at the diol, hot and concentrated it cleaves right through. A question that specifies KMnO₄ without conditions is incomplete, and one that specifies them is telling you which row to read.

What carries forward

Two threads. The syn/anti diol pair is a stereochemical choice you make by reagent, which is the same kind of control as Lindlar against dissolving metal in the last section — and both are the sort of thing a synthesis question is built around. And ozonolysis run backwards is a structure-determination technique, which puts it alongside the spectroscopy chapter rather than only alongside the reactions: given fragments, find the parent.